With regulated airguns, the relationship between the regulator's setpoint and the hammer spring tension is really quite simple. There is only one hammer spring setting for a given regulator setpoint that will yield the best consistency (extreme spread or standard deviation).
To find the optimal hammer spring setting, keep increasing the tension until the velocity no longer increases. Then back it off until the velocity is somewhere around 95% - 97% of that maximum. So for example, if your max velocity was 900fps, dial the hammer spring back until the velocity drops to about 855 - 873fps.
When adjusted in this manner, your airgun will be somewhat insensitive to the little inevitable variations in pressure or hammer strike. It is akin to how an unregulated PCP operates in and around the top of its bell curve (the sweet spot). It will also be reasonably efficient. Better efficiency would be possible by backing off the hammer spring tension further, but that puts the airgun operating at a state of partial valve lock. It will take little sips of air on each shot but the extreme spread suffers. For short range shooting (e.g. 10m practice in the basement), that may be fine....preferable, even. But it's no good for 50+ yards unless your accuracy standard is a soup can.
Accuracy on the other hand can't be so easily correlated to something as simple as the balance between regulator and hammer spring. Many, many things play into it. Having a stable velocity certainly helps but it's just one piece of the jigsaw puzzle.